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Dr. Erik A. Karlsson, Bao-Lin Lee, Dr. Torbjörn Åkermark, Eric V. Johnston, Markus D. Kärkäs, Dr. Junliang Sun, Dr. Örjan Hansson, Prof. Jan-E. Bäckvall and Prof. Björn Åkermark Photosensitized Water Oxidation by Use of a Bioinspired Manganese Catalyst Angewandte Chemie International Edition 50

Version of Record online: 7 OCT 2011 | DOI: 10.1002/anie.201104355

Thumbnail image of graphical abstract

Manganificent potential: A dinuclear manganese catalyst contains metal centers that are coordinated by a central phenolate, with adjoining imidazole and carboxylate groups, which are all important functionalities in the natural oxygen-evolving center. The complex catalyzes the conversion of water to oxygen in the presence of a single-electron oxidant [Ru(bpy)3]3+ (see picture, bpy=2,2′-bipyridine, A=acceptor).

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