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Christophe Das Neves Gomes, Dr. Olivier Jacquet, Dr. Claude Villiers, Dr. Pierre Thuéry, Dr. Michel Ephritikhine and Dr. Thibault Cantat A Diagonal Approach to Chemical Recycling of Carbon Dioxide: Organocatalytic Transformation for the Reductive Functionalization of CO2 Angewandte Chemie International Edition 51

Version of Record online: 29 SEP 2011 | DOI: 10.1002/anie.201105516

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Lateral thinking: A diagonal approach to CO2 recycling has been explored for the formation of both functionalized and energetic chemicals featuring a reduced carbon center. The strategy relies on the tandem use of a functionalization reagent and a reductant that can be independently modified to access a wide spectrum of chemicals from CO2. It is exemplified with an organocatalytic process to convert CO2 into formamides (see picture).

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