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Dr. Da-Peng Dong, Prof. Tao Liu, Dr. Shinji Kanegawa, Dr. Soonchul Kang, Prof. Osamu Sato, Prof. Cheng He and Prof. Chun-Ying Duan Photoswitchable Dynamic Magnetic Relaxation in a Well-Isolated {Fe2Co} Double-Zigzag Chain Angewandte Chemie International Edition 51

Version of Record online: 12 APR 2012 | DOI: 10.1002/anie.201105987

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Charge-transfer-induced spin transition occurs cooperatively and reversibly in the isolated FeIII2CoII chains of {[Fe(pzTp)(CN)3]2Co(4-styrylpyridine)2}⋅2 H2O ⋅2 CH3OH (1). When 1 is irradiated with 532 nm light, it shows single-chain magnetic behavior with no antiferromagnetic ordering after irradiation (see picture; C gray, N blue, B yellow; LS=low spin, HS=high spin).

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