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Philippe Berrouard, Dr. Ahmed Najari, Dr. Agnieszka Pron, David Gendron, Pierre-Olivier Morin, Jean-Rémi Pouliot, Justine Veilleux and Prof. Dr. Mario Leclerc Synthesis of 5-Alkyl[3,4-c]thienopyrrole-4,6-dione-Based Polymers by Direct Heteroarylation Angewandte Chemie International Edition 51

Article first published online: 11 NOV 2011 | DOI: 10.1002/anie.201106411

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Don't stand Stille: A direct heteroarylation polycondensation reaction was used for the synthesis of high-molecular-weight thienopyrroledione-based polymers (see scheme) in an impressive yield (up to 96 %) and in only a few synthetic steps. This new method is an alternative to the standard Stille coupling reaction and thus avoids formation of toxic tin by-products.

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