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Dr. Jingbo Chen, Jingchao Chen, Yan Xie and Prof. Dr. Hongbin Zhang Enantioselective Total Synthesis of (−)-Stenine Angewandte Chemie International Edition 51

Version of Record online: 16 DEC 2011 | DOI: 10.1002/anie.201106587

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In control: (−)-Stenine has been synthesized in 14 steps from commercially available compounds with an overall yield of 5.9 % by using a method that is based on double Michael addition. In the key step, the stereogenic centers that are required for (−)-stenine are generated in a highly stereocontrolled, asymmetric, one-pot cyclization to give a densely substituted cyclohexane core.

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