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Thomas Pauloehrl, Dr. Guillaume Delaittre, Volker Winkler, Dr. Alexander Welle, Dr. Michael Bruns, Prof. Dr. Hans G. Börner, Dr. Alexandra M. Greiner, Prof. Dr. Martin Bastmeyer and Prof. Dr. Christopher Barner-Kowollik Adding Spatial Control to Click Chemistry: Phototriggered Diels–Alder Surface (Bio)functionalization at Ambient Temperature Angewandte Chemie International Edition 51

Version of Record online: 9 DEC 2011 | DOI: 10.1002/anie.201107095

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A photoconjugation strategy based on light-triggered Diels–Alder addition of o-quinodimethanes is compatible with biomolecules and proceeds rapidly at ambient temperature without the need of a catalyst. Spatial control was confirmed by photopatterning of a small-molecule ATRP initiator, a polymer, and a peptide in a time-of-flight secondary-ion mass spectrometry investigation.

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