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Trung Cao, Joshua Deitch, Dr. Elizabeth C. Linton and Prof. Marisa C. Kozlowski Asymmetric Synthesis of Allenyl Oxindoles and Spirooxindoles by a Catalytic Enantioselective Saucy–Marbet Claisen Rearrangement Angewandte Chemie International Edition 51

Article first published online: 27 JAN 2012 | DOI: 10.1002/anie.201107417

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Saucy selection: The first catalytic, enantioselective Saucy–Marbet Claisen rearrangement has been achieved. Palladium(II) (R)-binap or tBuphox catalysts L*Pd(SbF6)2 were employed to generate allenyl oxindoles or spirolactones bearing a quaternary center with up to 98 % ee.

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