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Daniela Fuchs, Dr. Géraldine Rousseau, Dr. Lisa Diab, Urs Gellrich and Prof. Dr. Bernhard Breit Tandem Rhodium-Catalyzed Hydroformylation–Hydrogenation of Alkenes by Employing a Cooperative Ligand System Angewandte Chemie International Edition 51

Article first published online: 30 JAN 2012 | DOI: 10.1002/anie.201108946

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Dual action: A multifunctional rhodium catalyst system enables the simultaneous catalysis of two distinct transformations, hydroformylation of an alkene and reduction of an aldehyde, in a highly selective manner. This one-pot/two-step process is controlled by the cooperative action of two different supramolecular ligand systems and transforms terminal alkenes into C1-chain-elongated linear alcohols.

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