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Shunsuke Oishi and Dr. Susumu Saito Double Molecular Recognition with Aminoorganoboron Complexes: Selective Alcoholysis of β-Dicarbonyl Derivatives Angewandte Chemie International Edition 51

Version of Record online: 13 APR 2012 | DOI: 10.1002/anie.201200304

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Double duty: Aminoorganoboron (AOB) complexes recognize alcohol and β-dicarbonyl units, and thereby facilitate chemo- and site-selective alcoholysis of the latter (see scheme). The complex activates both reaction partners. This strategy enables C[BOND]C, C[BOND]N, and C[BOND]O bond cleavage in addition/elimination reactions under near neutral pH conditions and provides a new method for functional group conversions.

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