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Dr. Tia Jacobs, Dr. Gareth O. Lloyd, Dr. Jan-André Gertenbach, Prof. Kristian K. Müller-Nedebock, Prof. Catharine Esterhuysen and Prof. Leonard J. Barbour In Situ X-ray Structural Studies of a Flexible Host Responding to Incremental Gas Loading Angewandte Chemie International Edition 51

Version of Record online: 5 APR 2012 | DOI: 10.1002/anie.201201281

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Crystallographic pressure-lapse snapshots of a porous material responding to gas loading were used to investigate the stepwise uptake of carbon dioxide and acetylene molecules into discrete confined spaces. Based on the data, a qualitative statistical mechanical model was devised that reproduces even subtle features in the experimental gas sorption isotherms.

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