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Prof. Dr. Scott E. Denmark and Dr. Tyler W. Wilson Silyl Ketene Imines: Highly Versatile Nucleophiles for Catalytic, Asymmetric Synthesis Angewandte Chemie International Edition 51

Version of Record online: 11 SEP 2012 | DOI: 10.1002/anie.201202139

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Teaching a middled-aged nucleophile new tricks: This Minireview provides an overview on the development of silyl ketene imines and their recent applications in catalytic, enantioselective reactions. The unique structure of ketene imines allow a diverse range of reactivity patterns and provide solutions to existing challenges in the enantioselective construction of quaternary stereogenic carbon centers and cross-benzoin adducts (see scheme; Pg=protecting group, Y=OPg).

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