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Dr. Brett P. Fors and Prof. Dr. Craig J. Hawker Control of a Living Radical Polymerization of Methacrylates by Light Angewandte Chemie International Edition 51

Article first published online: 13 JUL 2012 | DOI: 10.1002/anie.201203639

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On–off: A living radical polymerization procedure, which utilizes ppm levels of an iridium-based photoredox catalyst, affords control over chain growth through mediation by visible light (see scheme; Pn=polymer chain, X=halogen, M=monomer). This process can be activated and deactivated by light, enables control over the molecular weight and molecular weight distributions, and tolerates different functional groups.

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