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Fezile Lakadamyali, Dr. Masaru Kato, Dr. Nicoleta M. Muresan and Dr. Erwin Reisner Selective Reduction of Aqueous Protons to Hydrogen with a Synthetic Cobaloxime Catalyst in the Presence of Atmospheric Oxygen Angewandte Chemie International Edition 51

Version of Record online: 22 AUG 2012 | DOI: 10.1002/anie.201204180

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Protons preferred: A cobalt catalyst is reported that evolves H2 electro- and photocatalytically at room temperature, in pH-neutral water, and in the presence of atmospheric O2 (see scheme). The catalyst shows respectable Faradaic efficiencies under N2 and 21 % O2 in N2, and can be used under both homogeneous and heterogeneous conditions.

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