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Dr. Jier Huang, Onur Buyukcakir, Michael W. Mara, Dr. Ali Coskun, Dr. Nada M. Dimitrijevic, Gokhan Barin, Dr. Oleksandr Kokhan, Dr. Andrew B. Stickrath, Dr. Romain Ruppert, Dr. David M. Tiede, Prof. J. Fraser Stoddart, Prof. Jean-Pierre Sauvage and Prof. Lin X. Chen Highly Efficient Ultrafast Electron Injection from the Singlet MLCT Excited State of Copper(I) Diimine Complexes to TiO2 Nanoparticles Angewandte Chemie International Edition 51

Version of Record online: 8 NOV 2012 | DOI: 10.1002/anie.201204341

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Cu complexes as photosensitizers: Photoinduced charge-transfer dynamics from a copper(I) diimine complex to TiO2 nanoparticles were investigated by combining multiple time-resolved spectroscopic methods. An efficient and ultrafast electron transfer process from the singlet MLCT state was discovered as a result of structural control owing to the flattening of the tetrahedral geometry in the complex and the bulky groups in the ligands.

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