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Dr. Saeed Kamali, Dr. Hongxin Wang, Dr. Devrani Mitra, Dr. Hideaki Ogata, Prof. Wolfgang Lubitz, Brian C. Manor, Prof. Thomas B. Rauchfuss, Dr. Deborah Byrne, Dr. Violaine Bonnefoy, Prof. Francis E. Jenney Jr., Prof. Michael W. W. Adams, Dr. Yoshitaka Yoda, Dr. Ercan Alp, Dr. Jiyong Zhao and Prof. Stephen P. Cramer Observation of the Fe[BOND]CN and Fe[BOND]CO Vibrations in the Active Site of [NiFe] Hydrogenase by Nuclear Resonance Vibrational Spectroscopy Angewandte Chemie International Edition 52

Version of Record online: 8 NOV 2012 | DOI: 10.1002/anie.201204616

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Nuclear inelastic scattering of 57Fe labeled [NiFe] hydrogenase is shown to give information on different states of the enzyme. It was thus possible to detect and assign Fe[BOND]CO and Fe[BOND]CN bending and stretching vibrations of the active site outside the spectral range of the Fe[BOND]S cluster normal modes.

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