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Prof. Dr. Kazuhiko Maeda and Prof. Dr. Kazunari Domen Water Oxidation Using a Particulate BaZrO3-BaTaO2N Solid-Solution Photocatalyst That Operates under a Wide Range of Visible Light Angewandte Chemie International Edition 51

Version of Record online: 5 SEP 2012 | DOI: 10.1002/anie.201204635

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Tripping the light fantastic: Despite small band gap energies (1.7–1.8 eV), BaZrO3-BaTaO2N solid solutions (Zr/Ta≤0.1) are capable of photocatalyzing both water oxidation and reduction even under irradiation above 660 nm. Solar water splitting to form H2 and O2 was also demonstrated using a photoelectrochemical cell consisting of a BaZrO3–BaTaO2N solid solution as an anode and a Pt wire cathode.

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