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Yuki Hoshino, Yu Shibata and Prof. Dr. Ken Tanaka Rhodium-Catalyzed Three-Component Cross-Addition of Silylacetylenes, Alkynyl Esters, and Electron-Deficient Alkenes or Isocyanates Angewandte Chemie International Edition 51

Article first published online: 21 AUG 2012 | DOI: 10.1002/anie.201204646

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‘Rh'oad crossing: A cationic RhI/(cod)2 complex catalyzes the chemo-, regio-, and stereoselective title reaction with electron-deficient alkenes leading to substituted 1,3-dienes. The analogous three-component cross-addition involving isocyanates instead of alkenes has also been developed.

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