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Agnieszka Adamska, Dr. Alexey Silakov, Dr. Camilla Lambertz, Dr. Olaf Rüdiger, Prof. Thomas Happe, Dr. Edward Reijerse and Prof. Wolfgang Lubitz Identification and Characterization of the “Super-Reduced” State of the H-Cluster in [FeFe] Hydrogenase: A New Building Block for the Catalytic Cycle? Angewandte Chemie International Edition 51

Version of Record online: 26 OCT 2012 | DOI: 10.1002/anie.201204800

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Super-reduced and super-active: A new redox state in the active site of algal [FeFe] hydrogenases has been identified and characterized by EPR and FTIR spectroscopy. Electrochemical and in vitro essays show that this species is highly active in hydrogen production and suggest that it is a key intermediate in the catalytic cycle of all [FeFe] hydrogenases.

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