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Prof. Dr. Wolfgang Buckel, Dr. Peter Friedrich and Prof. Dr. Bernard T. Golding Hydrogen Bonds Guide the Short-Lived 5′-Deoxyadenosyl Radical to the Place of Action Angewandte Chemie International Edition 51

Version of Record online: 3 SEP 2012 | DOI: 10.1002/anie.201205299

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Radical chaperone: Recent research reveals how the 5′-deoxyadenosyl radical (see structure) is generated by homolysis of the Co[BOND]C σ-bond of enzyme-bound coenzyme B12 and how it is guided to the substrate through pseudorotation of the ribose moiety and hydrogen-bonding interactions.

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