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Dr. Aliaksandr S. Bandarenka, Ana Sofia Varela, Mohammedreza Karamad, Dr. Federico Calle-Vallejo, Dr. Lone Bech, Dr. Francisco J. Perez-Alonso, Dr. Jan Rossmeisl, Dr. Ifan E. L. Stephens and Prof. Ib Chorkendorff Design of an Active Site towards Optimal Electrocatalysis: Overlayers, Surface Alloys and Near-Surface Alloys of Cu/Pt(111) Angewandte Chemie International Edition 51

Version of Record online: 22 OCT 2012 | DOI: 10.1002/anie.201205314

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I could never be without Cu: An active site has been designed for the catalysis of CO electroxidation. This was achieved by incorporating submonolayer amounts of Cu (orange spheres) into a single crystal of Pt (gray spheres). The electrochemical reactivity of this surface was highly sensitive to the exact position of Cu (see scheme).

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