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Xiaoyu Chen, Dr. Xingyong Wang, Dr. Yunxia Sui, Prof. Yizhi Li, Prof. Jing Ma, Prof. Jinglin Zuo and Prof. Xinping Wang Synthesis, Characterization, and Structures of a Persistent Aniline Radical Cation Angewandte Chemie International Edition 51

Version of Record online: 18 OCT 2012 | DOI: 10.1002/anie.201205478

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Feeling the heat: The aniline radical cation TBA.+ (TBA=2,4,6-tBu3C6H2NH2) has been successfully stabilized both in solution and in the solid state. It exists as two isomers in the crystal lattice that interchange with temperature, and features an exceptionally long C[BOND]N bond beyond theoretical prediction.

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