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Prof. Angiolina Comotti, Dr. Silvia Bracco, Martino Mauri, Sergio Mottadelli, Prof. Teng Ben, Prof. Shilun Qiu and Prof. Piero Sozzani Confined Polymerization in Porous Organic Frameworks with an Ultrahigh Surface Area Angewandte Chemie International Edition 51

Article first published online: 5 SEP 2012 | DOI: 10.1002/anie.201205618

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Polymers framed: Interpenetrated nanocomposites were formed by polymerization of acrylonitrile in a ultrahigh surface area (>5000 m2 g−1) porous framework. The resulting material realizes a hyperextended interface with uniform interdigitation of the two structures at the size limit of the individual molecular moieties. The confined poly(acrylonitrile) chains could be transformed into light-absorbing polyconjugated ladder polymers.

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