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Jaeyune Ryu, Kwangmin Shin, Sae Hume Park, Ji Young Kim and Prof. Dr. Sukbok Chang Rhodium-Catalyzed Direct C[BOND]H Amination of Benzamides with Aryl Azides: A Synthetic Route to Diarylamines Angewandte Chemie International Edition 51

Article first published online: 31 AUG 2012 | DOI: 10.1002/anie.201205723

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No muss, no fuss: A rhodium-catalyzed direct intermolecular C[BOND]H amination of benzamides and ketoximes using aryl azides as the amine source has been developed. The reaction exhibits a broad substrate scope with excellent functional-group tolerance, requires no external oxidants, releases N2 as the only by-product, and produces diarylamines in high yields.

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