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Dr. Wenju Zhu, Jie Fang, Yong Liu, Jun Ren and Prof. Zhongwen Wang Lewis Acid Catalyzed Formal Intramolecular [3+2] Cross-Cycloaddition of Cyclopropane 1,1-Diesters with Alkenes: General and Efficient Strategy for Construction of Bridged [n.2.1] Carbocyclic Skeletons Angewandte Chemie International Edition 52

Version of Record online: 10 JAN 2013 | DOI: 10.1002/anie.201206484

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Carbon bridges: The title reaction has been successfully developed, and applied to the total synthesis of the tetracyclic diterpenoids phyllocladanol and phyllocladene. The method provides an efficient, general, and conceptually new strategy for the construction of structurally complex and diverse [n.2.1] carbocyclic skeletons (see scheme).

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