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Katharina Schwinghammer, Brian Tuffy, Maria B. Mesch, Eva Wirnhier, Charlotte Martineau, Prof. Francis Taulelle, Prof. Wolfgang Schnick, Prof. Jürgen Senker and Prof. Bettina V. Lotsch Triazine-based Carbon Nitrides for Visible-Light-Driven Hydrogen Evolution Angewandte Chemie International Edition 52

Version of Record online: 22 JAN 2013 | DOI: 10.1002/anie.201206817

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A new dimension: The doping of amorphous poly(triazine imide) (PTI) through ionothermal copolymerization of dicyandiamide with 4-amino-2,6-dihydroxypyrimidine (4AP) results in triazine-based carbon nitrides with increased photoactivity for water splitting compared to crystalline poly(triazine imide) (PTI/Li+Cl, see picture) and melon-type carbon nitrides. This family of carbon nitride semiconductors has potential as low-cost, environmentally clean photocatalysts for solar fuel production.

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