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Dr. Takashi Kamegawa, Sachiyo Matsuura, Hiroki Seto and Prof. Dr. Hiromi Yamashita A Visible-Light-Harvesting Assembly with a Sulfocalixarene Linker between Dyes and a Pt-TiO2 Photocatalyst Angewandte Chemie International Edition 52

Version of Record online: 29 NOV 2012 | DOI: 10.1002/anie.201206839

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Successful anchoring of cationic dye molecules (thiazole orange, TO) on Pt-TiO2 for a visible-light-harvesting assembly was achieved by surface modification of Pt-TiO2 with 4-sulfocalix[4]arene as a linker, leading to formation of surface complexes (see picture). This heterogeneous system can act as an efficient photocatalyst for production of hydrogen in the presence of a sacrificial reagent (TEOA=triethanolamine).

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