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Dr. Kenneth Hanson, Daniel A. Torelli, Dr. Aaron K. Vannucci, Dr. M. Kyle Brennaman, Hanlin Luo, Dr. Leila Alibabaei, Dr. Wenjing Song, Dennis L. Ashford, Michael R. Norris, Dr. Christopher R. K. Glasson, Dr. Javier J. Concepcion and Prof. Thomas J. Meyer Self-Assembled Bilayer Films of Ruthenium(II)/Polypyridyl Complexes through Layer-by-Layer Deposition on Nanostructured Metal Oxides Angewandte Chemie International Edition 51

Article first published online: 9 NOV 2012 | DOI: 10.1002/anie.201206882

Thumbnail image of graphical abstract

Simple assembly: A “layer-by-layer” deposition of functionalized dyes/catalysts on the surfaces of nanocrystalline oxides is introduced. The strategy is general and offers considerable flexibility based on phosphonate- or carboxylate-binding groups with ZrIV as bridging ions. The resulting bilayer structures are capable of supporting rapid intra-layer energy and electron transfer (see picture).

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