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Dr. Ganglong Cui and Prof. Dr. Walter Thiel Photoinduced Ultrafast Wolff Rearrangement: A Non-Adiabatic Dynamics Perspective Angewandte Chemie International Edition 52

Version of Record online: 4 DEC 2012 | DOI: 10.1002/anie.201207628

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One reaction, two routes: Full-dimensional non-adiabatic dynamics simulations shed light on the ultrafast photoinduced Wolff rearrangement in an α-diazocarbonyl compound. The trajectories show both concerted asynchronous and stepwise processes leading to the corresponding ketene (see scheme).

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