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P. Alex Rudd, Shengsi Liu, Dr. Nora Planas, Dr. Eckhard Bill, Prof. Dr. Laura Gagliardi and Prof. Dr. Connie C. Lu Multiple Metal–Metal Bonds in Iron–Chromium Complexes Angewandte Chemie International Edition 52

Version of Record online: 11 MAR 2013 | DOI: 10.1002/anie.201208686

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Mix and match: The first structural examples of M[BOND]M multiple bonds between different first-row transition metals are elucidated using X-ray crystallography (see picture; Fe pink, Cr green, P yellow, N blue), spectroscopic methods, and calculations. The Fe[BOND]Cr bonds are ultrashort (<2 Å) with highly delocalized σ and π bonds and unusually large quadrupole splittings in Mössbauer spectroscopy.

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