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Dr. Youqian Deng and Prof. Dr. Jan-E. Bäckvall Palladium-Catalyzed Oxidative Acyloxylation/Carbocyclization of Allenynes Angewandte Chemie International Edition 52

Article first published online: 5 FEB 2013 | DOI: 10.1002/anie.201208718

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New bonds: The title reaction provides access to synthetically useful acyloxylated vinylallenes where a new C[BOND]C bond, a new C[BOND]O bond, and a new allene structure are formed. Furthermore, an aerobic version of this transformation was realized using catalytic amounts of p-benzoquinone (BQ) together with catalytic amounts of cobalt salophen.

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