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Zhao-Lin He, Huai-Long Teng and Prof. Dr. Chun-Jiang Wang Fulvenes as Effective Dipolarophiles in Copper(I)-Catalyzed [6+3] Cycloaddition of Azomethine Ylides: Asymmetric Construction of Piperidine Derivatives Angewandte Chemie International Edition 52

Version of Record online: 30 JAN 2013 | DOI: 10.1002/anie.201208799

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As easy as π: Fulvenes serve as 6π dipolarophiles in the title reaction in the presence of the chiral CuI/(S)-L complex. The present system provides a unique and straightforward access to enantioenriched, highly functionalized piperidine derivatives in good yields and excellent diastereoselectivities and enantioselectivities.

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