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Hongwei Zhang, Weiya Pu, Dr. Tao Xiong, Dr. Yan Li, Xue Zhou, Kai Sun, Prof. Dr. Qun Liu and Prof. Dr. Qian Zhang Copper-Catalyzed Intermolecular Aminocyanation and Diamination of Alkenes Angewandte Chemie International Edition 52

Version of Record online: 25 JAN 2013 | DOI: 10.1002/anie.201209142

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′N′ front and center: The facile construction of C[BOND]N bonds by the generation of nitrogen-centred radicals from N-fluorobenzenesulfonimide results in the aminative difuctionalization of alkenes. The first copper-catalyzed intermolecular aminocyanation of alkenes and diamination of styrenes were realized. Si–F and B–F interactions play a significant role in the reaction.

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