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Yusuke Izawa, Dr. Changwu Zheng and Prof. Shannon S. Stahl Aerobic Oxidative Heck/Dehydrogenation Reactions of Cyclohexenones: Efficient Access to meta-Substituted Phenols Angewandte Chemie International Edition 52

Version of Record online: 19 FEB 2013 | DOI: 10.1002/anie.201209457

Thumbnail image of graphical abstract

Jockeying for the (meta)position: A new dicationic palladium(II) catalyst, employing a 6,6′-dimethyl-2,2′-bipyridine ligand, promotes both the aerobic oxidative Heck coupling and dehydrogenation reactions of cyclohexenones. These reactions may be combined in a one-pot sequence to enable the straightforward synthesis of meta-substituted phenols (see scheme).

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