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Prof. Dr. Mukund P. Sibi and Prof. Dr. Yannick Landais C sp 3[BOND]F Bond Formation: A Free-Radical Approach Angewandte Chemie International Edition 52

Article first published online: 25 FEB 2013 | DOI: 10.1002/anie.201209583

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Totally rad: Synthetic methods have been developed for the formation of Csp3[BOND]F bonds by reaction of C-centered radicals with fluorine sources. Three complementary strategies, which differ in the mode of generation of the alkyl radical intermediate, are described. These include olefin hydrofluorination, decarboxylative fluorination, and aliphatic C[BOND]H fluorination.

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