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Dr. Li-Mei Jin, Dr. Xue Xu, Dr. Hongjian Lu, Dr. Xin Cui, Dr. Lukasz Wojtas and Prof. Dr. X. Peter Zhang Effective Synthesis of Chiral N-Fluoroaryl Aziridines through Enantioselective Aziridination of Alkenes with Fluoroaryl Azides Angewandte Chemie International Edition 52

Version of Record online: 15 APR 2013 | DOI: 10.1002/anie.201209599

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The CoII complex of a D2-symmetric chiral porphyrin ([Co(D2-Por*)], see scheme) is a highly effective catalyst for the enantioselective aziridination of alkenes with fluoroaryl azides. The reaction can be performed at RT with low catalyst loading, and the olefin is the limiting reagent. Furthermore, the reaction is tolerant toward different combinations of aromatic olefins and fluoroaryl azides.

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