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Dr. Hun Young Kim, Jian-Yuan Li and Prof. Dr. Kyungsoo Oh A Soft Vinyl Enolization Approach to α-Acylvinyl Anions: Direct Aldol/Aldol Condensation Reactions of (E)-β-Chlorovinyl Ketones Angewandte Chemie International Edition 52

Article first published online: 18 FEB 2013 | DOI: 10.1002/anie.201209876

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Synthesizing the synthons: The development of α-acylvinyl anion synthons has been achieved using direct α-vinyl enolization of α,β-unsaturated ketones under mild reaction conditions. The synthetic utility of such synthons has been demonstrated in intermolecular aldol and aldol condensation reactions, which provide synthetically useful allenyl ketone and enyne derivatives.

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