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Dr. Robert Kretschmer, Dr. Maria Schlangen and Prof. Dr. Helmut Schwarz Isomer-Selective Thermal Activation of Methane in the Gas Phase by [HMO]+ and [M(OH)]+ (M=Ti and V) Angewandte Chemie International Edition 52

Version of Record online: 25 APR 2013 | DOI: 10.1002/anie.201300900

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Methane scrabble: To have the right elements is sometimes just not sufficient, as shown by [M(OH)]+ (M=Ti, V), which do not react with methane. However, reshuffling of the “tiles” to [HMO]+ changes the reactions behavior completely, leading to the first example of C[BOND]H bond activation of methane by an early first-row transition-metal cation.

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