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Ziwei Tang, Xiaowei Chen, Hao Chen, Prof. Limin Wu and Prof. Xuebin Yu Metal-Free Catalysis of Ammonia–Borane Dehydrogenation/Regeneration for a Highly Efficient and Facilely Recyclable Hydrogen-Storage Material Angewandte Chemie International Edition 52

Version of Record online: 22 APR 2013 | DOI: 10.1002/anie.201301049

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As easy as ABC: Mesoporous graphitic carbon nitride (MGCN; g-C3N4) is utilized to support ammonia borane (AB) on the basis of its accessible nanoporous structure and basic properties. A high loading of uniformly dispersed AB nanoparticles into the MGCN is possible giving greatly enhanced H2 generation from AB, and facile regeneration cycles by a hydrazine hydrogenation process, even at room temperature.

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