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Yu Sun, Ruofan Li, Wenhao Zhang and Prof. Dr. Ang Li Total Synthesis of Indotertine A and Drimentines A, F, and G Angewandte Chemie International Edition 52

Version of Record online: 15 JUL 2013 | DOI: 10.1002/anie.201303334

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Oh my darling, Drimentine: The first total synthesis of the pyrroloindoline alkaloids drimentines A, F, and G, and their congener, indotertine A, is reported. An intermolecular radical conjugate addition was key in the synthesis of the drimentine alkaloids, and a biologically inspired iminium–olefin cyclization converted drimentine F into indotertine A.

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