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Dr. Victor Mougel, Lucile Chatelain, Dr. Johannes Hermle, Dr. Roberto Caciuffo, Dr. Eric Colineau, Dr. Floriana Tuna, Dr. Nicola Magnani, Dr. Arnaud de Geyer, Dr. Jacques Pécaut and Dr. Marinella Mazzanti A Uranium-Based UO2+–Mn2+ Single-Chain Magnet Assembled trough Cation–Cation Interactions Angewandte Chemie International Edition 53

Version of Record online: 6 DEC 2013 | DOI: 10.1002/anie.201307366

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Uranium in chains: 5f–3d heterometallic 1D chains are assembled from the reaction of pentavalent uranyl and CdII or MnII. The Mn-UO2-Mn coordination polymer exhibits slow relaxation of magnetization with a high relaxation barrier, and shows an open hysteresis cycle, thus affording the first example of an actinide-based single-chain magnet.

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