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Dr. Eric Gouré, Dr. Frédéric Avenier, Patrick Dubourdeaux, Dr. Olivier Sénèque, Dr. Florian Albrieux, Colette Lebrun, Dr. Martin Clémancey, Dr. Pascale Maldivi and Dr. Jean-Marc Latour A Diiron(III,IV) Imido Species Very Active in Nitrene-Transfer Reactions Angewandte Chemie International Edition 53

Version of Record online: 13 JAN 2014 | DOI: 10.1002/anie.201307429

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Nitrene transfer: An FeIIIFeIV imido intermediate is identified in nitrene-transfer reactions by desorption electrospray ionization mass spectrometry (DESI-MS). DFT calculations show that low-lying FeIIIFeIII-.N-tosyl configurations play a major role in the high reactivity of the intermediate.

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