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Sina Schwendemann, Shunsuke Oishi, Prof. Dr. Susumu Saito, Dr. Roland Fröhlich, Dr. Gerald Kehr and Prof. Dr. Gerhard Erker Reaction of an “Invisible” Frustrated N/B Lewis Pair with Dihydrogen Chemistry – An Asian Journal 8

Version of Record online: 25 OCT 2012 | DOI: 10.1002/asia.201200776

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I′m frustrated—why do I seem so invisible to you: Piers' borane [HB(C6F5)2] forms a Lewis acid/Lewis base adduct B with the enamine A. This reacts with dihydrogen via the “invisible” frustrated N/B Lewis pair C, probably formed by means of hydroboration under equilibrium conditions, to yield the zwitterionic ammonium/hydrido-borate product D.

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