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Rui Zhang, Dr. Danmeng Shuai, Dr. Kathryn A. Guy, Prof. John R. Shapley, Prof. Timothy J. Strathmann and Prof. Charles J. Werth Elucidation of Nitrate Reduction Mechanisms on a Pd-In Bimetallic Catalyst using Isotope Labeled Nitrogen Species ChemCatChem 5

Version of Record online: 23 NOV 2012 | DOI: 10.1002/cctc.201200457

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A game of tag: 15N-labeling is shown to be an effective tool for the study of the nitrate/nitrite reduction pathways by eliminating interference from atmospheric 14N2. A new kinetic model is proposed, which indicates that highly reactive adsorbed NO (NO*), or other unspecified adsorbed N species, is a key intermediate involved in determining final product selectivity.

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