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Weijia Gan, Dr. Dennis J. M. Snelders, Prof. Paul J. Dyson and Prof. Gábor Laurenczy Ruthenium(II)-Catalyzed Hydrogen Generation from Formic Acid using Cationic, Ammoniomethyl-Substituted Triarylphosphine Ligands ChemCatChem 5

Article first published online: 13 MAR 2013 | DOI: 10.1002/cctc.201200782

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Proceed with cation: New RuII catalysts for aqueous-phase HCOOH decomposition into H2 and CO2 that use a series of oligocationic, ammoniomethyl-substituted triarylphosphine ligands are developed. Excellent activities are achieved, that is, TOFs of 1950 h−1 and TONs of over 10 000.

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