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Dr. Zheng Xu, Nicholas D. McNamara, Gregory T. Neumann, Prof. William F. Schneider and Prof. Jason C. Hicks Catalytic Hydrogenation of CO2 to Formic Acid with Silica-Tethered Iridium Catalysts ChemCatChem 5

Version of Record online: 11 APR 2013 | DOI: 10.1002/cctc.201200839

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Tetherball: A heterogeneous, mesoporous silica-tethered iridium catalyst (Ir-PN/SBA-15) containing a bidentate iminophosphine ligand is synthesized for the hydrogenation of CO2 to formic acid in aqueous solution. This new recyclable catalyst exhibits high activities to formic acid production under mild conditions [60 °C, 4.0 MPa total pressure (H2/CO2=1:1)].

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