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Dr. Jean-Baptiste Sortais and Prof. Dr. Christophe Darcel Chiral Cyclopentadienyl-type Ligands: a New Breakthrough for Asymmetric C[BOND]H Functionalisation ChemCatChem 5

Version of Record online: 7 MAR 2013 | DOI: 10.1002/cctc.201200874

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Ligand breakthrough: Using a well-designed chiral cyclopentadienyl rhodium complex as the catalyst, an efficient asymmetric C[BOND]H bond functionalization/cyclization was performed at RT in the presence of a catalytic amount of dibenzoylperoxide (DBPO) leading to tetrahydroiso-quinolinone derivatives with moderate to good yields and very good enantiomeric ratios.

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