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Dr. Senthil Narayanaperumal, Prof. Daniel G. Rivera, Rodrigo C. Silva and Prof. Márcio W. Paixão Terpene-Derived Bifunctional Thioureas in Asymmetric Organocatalysis ChemCatChem 5

Article first published online: 15 APR 2013 | DOI: 10.1002/cctc.201200936

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From pine resin to catalyst: The easily available rosin diterpene abietic acid has been transformed into a unique class of bifunctional thiourea catalysts that can also incorporate further substituents, thereby enabling either Lewis base or enamine activation modes. Their application in a wide range of stereoselective transformations has revealed the positive effect of this chiral and rigid skeleton on the catalytic performance of these hybrid thioureas.

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