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Zhenzhen Kang, Guoyong Fang, Qingping Ke, Jianbo Hu and Prof. Dr. Tiandi Tang Superior Catalytic Performance of Mesoporous Zeolite TS-1 for the Oxidation of Bulky Organic Sulfides ChemCatChem 5

Version of Record online: 2 APR 2013 | DOI: 10.1002/cctc.201300084

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Rich man, pore man: A facile and universal route to mesoporous zeolite TS-1 (MTS-1) is reported. Compared with mesoporous-free TS-1, the MTS-1 zeolite shows extraordinarily catalytic activity and highly controllable chemoselectivity for the oxidation of sulfides into sulfoxides or sulfones. Based on the catalytic data, the Ti[BOND]hydroperoxo (η2) group is proposed to be the active site for the oxidation of sulfides into sulfoxides and sulfones.

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