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Yuanyuan Dong, Shouying Huang, Dr. Shengping Wang, Dr. Yujun Zhao, Prof. Dr. Jinlong Gong and Prof. Dr. Xinbin Ma Synthesis of Dimethyl Carbonate through Vapor-Phase Carbonylation Catalyzed by Pd-Doped Zeolites: Interaction of Lewis Acidic Sites and Pd Species ChemCatChem 5

Article first published online: 11 JUN 2013 | DOI: 10.1002/cctc.201300170

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All doped up: The interaction between Lewis (L) acidic sites and Pd species in the vapor-phase carbonylation reaction of methyl nitrite over Pd/Faujasite (FAU) catalysts is determined quantitatively. By keeping the Pd species in an electron-deficient state, the Lewis acids of the Pd/FAU catalysts promote the synthesis of dialkyl carbonates.

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