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Katerina Sordakis, Prof. Matthias Beller and Prof. Gábor Laurenczy Chemical Equilibria in Formic Acid/Amine-CO2 Cycles under Isochoric Conditions using a Ruthenium(II) 1,2-Bis(diphenylphosphino)ethane Catalyst ChemCatChem 6

Version of Record online: 7 NOV 2013 | DOI: 10.1002/cctc.201300740

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FA-ntastic! The equilibrium position in formic acid (FA)/amine–CO2 systems is examined as a function of pressure and temperature. High yields of FA dehydrogenation into H2 and CO2 are favored at low pressures and/or high temperatures, and H2 uptake is possible at elevated gas pressures, which takes us one step closer to the realization of a practical H2 storage–discharge device.

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